Angrand's Impressionist paintings of the early 1880s, generally depicting rural subjects and containing broken brushstrokes and light-filled colouration, reflect the influences of Claude Monet, Camille Pissarro, and Jules Bastien-Lepage. Through his interactions with Seurat, Signac, and others in the mid-1880s, his style evolved towards Neo-Impressionism. From 1887 his paintings were Neo-Impressionist and his drawings incorporated Seurat's tenebrist style. Angrand had the "ability to distil poetry from the most banal suburban scene". In 1887 he met van Gogh, who proposed a painting exchange (which ultimately did not happen). Van Gogh was influenced by Angrand's thick brushstrokes and Japanese-inspired compositional asymmetry. Also in 1887, "L'Accident", his first Divisionist painting, was exhibited at the Salon des Indépendants. Angrand joined Seurat in plein air painting on La Grande Jatte island.