In 1966, Berger co-starred with Kirk Douglas in the film "Cast a Giant Shadow". Berger played the role of Magda, a soldier in the Israeli army during the 1947–1949 Palestine war (1948). Also in 1966, the British film "Our Man in Marrakesh", called "Bang, Bang, You're Dead" in the U.S., was released, starring Senta Berger opposite Tony Randall. In "The Quiller Memorandum", a third film of hers released in 1966, she played opposite Max von Sydow and George Segal in the role of a German schoolteacher involved in neo-Nazi activity. In 1967, Berger acted in the pilot film for the Robert Wagner television series "It Takes a Thief", which aired on American television network ABC on 9 January 1968. She reprised her role in the series in October 1969, in an episode in which her character was killed off.