In 1960, Moore commenced recording sessions with Presley at RCA Victor and also served as production manager at Sam Phillips Recording Service, which involved supervising all aspects of studio operation. Moore played on such Presley songs as "Fame and Fortune", "Such a Night", "Frankfort Special", "Surrender", "I Feel So Bad", "Rock-a-Hula Baby", "Kiss Me Quick", "Good Luck Charm", "She's Not You", "(You're the) Devil in Disguise", and "Bossa Nova Baby". Moore remained as a guitarist for the majority of songs recorded after Presley's work was dominated by Hollywood sessions. He mostly played rhythm guitar however, with his last lead guitar work occurring by 1962 with "(You're the) Devil in Disguise". Moore also played on sessions for Roy Orbison (most notably on “Crying”) and others.