Azaria played Gargamel in the computer-animated/live-action adaptation of "The Smurfs" (2011). Azaria wore a prosthetic nose, ears, buck teeth, eyebrows and a wig, as well as shaving his head. He spent approximately 130 hours in the make-up chair over the course of the production. Azaria considered Gargamel's voice to be the most important part of his performance. The producers wanted an "old, failed, Shakespearean actor" voice, but Azaria felt this would lack energy and wanted something more Eastern European. He eventually selected a voice similar to that of Paul Winchell's from the cartoon. Azaria disliked the cartoon when it first aired, and considered Gargamel too one-dimensional a character and "just this straight villain"; he opted to make Gargamel "more sarcastic" than in the cartoon, but "discovered that there's no way to play Gargamel without screaming your head off at certain points – ramping him up and getting him very upset over Smurfs". He interpreted him as "very lonely", adding that "he hates the Smurfs because they're such a happy family. He wants in really badly. I think he wants to be embraced as a Smurf". Azaria worked with the writers to "infuse" the script with some of his ideas about the character, "particularly with the 'married' relationship between Gargamel and cat Azreal " which Azaria conceived.