For the BBC Learning project "Off By Heart Shakespeare", Walters delivered one of Shakespeare's best known speeches — "But soft, what light through yonder window breaks?" from "Romeo and Juliet". In October 2011, Walters starred in the Arjun Rose slasher "Demons Never Die". From 31 October 2011, he played Dushane in Channel 4's four-part drama "Top Boy". In February 2012, he played Chris in the BBC drama "Inside Men". In 2013, Walters reprised his role as main character Dushane in the second series of "Top Boy".