In May, in the qualification to the Brussels Open, Larcher de Brito won in the first qualifying round over Alicja Rosolska. In the second round, she lost to Yulia Putintseva. Later, she failed to qualify to the main draw at the French Open, where she lost in the first round of the qualifying to Maryna Zanevska. In June, playing in the qualifying phase at Birmingham, Larcher de Brito lost in the first qualifying round to Arantxa Parra Santonja. At Wimbledon, she qualified for the main draw by defeating Chanel Simmonds, Claire Feuerstein and Shahar Pe'er. In the first round of the main draw, Larcher de Brito defeated Melanie Oudin in three sets. In the second round, she defeated 2004 champion and world No. 3 Maria Sharapova in straight sets. In the third round, however, she lost to the unseeded Karin Knapp from Italy.