Since 2011, Denisof has been relatively active. He played a voice role in the animated DC movie '. He was featured in the majority of episodes in the AOL webseries, "Little Women, Big Cars". Denisof was then cast as a lead in Bryan Singer's new webseries '. He then reunited with Joss Whedon for two different film projects. The first was a minor role in the summer blockbuster "The Avengers", as The Other, a servant of the character Thanos, and a cohort of Loki. The second was the lead male role in a modern version of Shakespeare's "Much Ado About Nothing", which premiered at the Toronto Film Festival, to positive reviews from critics. The film was released worldwide in June 2013.