In 2010 he played Louis Zabel in Oliver Stone's "" alongside Michael Douglas, Shia LaBeouf, and Carey Mulligan. That same year he played a supporting role in "All Good Things" alongside Ryan Gosling and Kirsten Dunst. In 2011, Langella starred in the drama thriller "Unknown" alongside Liam Neeson and Diane Kruger. In 2012, he earned critical praise for his role in the independent film "Robot & Frank" with Peter Travers of Rolling Stone magazine calling his performance "a masterclass in acting".