In April 1907, Taylor married Sydney-born artist, inventor, and craftworker George Augustine Taylor at St Stephen's Presbyterian Church in Sydney. George Taylor had lectured her at college and was a close friend of her first employer Francis Ernest Stowe. On 5 December 1909, Taylor became the first Australian woman to fly a heavier-than-air craft, in a glider built by her husband in his Redfern workshop, from the Narrabeen sandhills near Sydney. They were both passionate about architecture and town planning, amongst many other interests and activities. Max Freeland described them as "possibly the most amazing couple in Australia's history".