As a result of his World Cup performances, Gilberto garnered a move to the Premier League to sign for Arsenal that summer for a fee of £4.5 million. During his six years at Arsenal, Gilberto gained a reputation as one of the best defensive midfielders in the world, and starred in a midfield duo alongside Patrick Vieira. He would feature as a member of the "Invincibles", where he captured his first top-flight league title as his team went undefeated the whole season, as well as winning two FA Cups. Gilberto also holds distinct records at Arsenal, recording their first goal at the Emirates Stadium, as well as their fastest ever goal, scoring in 21 seconds from kickoff against PSV Eindhoven in the 2002–03 UEFA Champions League. After departing Arsenal, Gilberto relocated to Greece, playing for Panathinaikos, where he won a domestic double. He then returned to Brazil in 2011, signing for Grêmio, where he remained for two years, before returning to Atlético to win the 2013 Copa Libertadores prior to retiring.