The new millennium saw the release of two recordings: "Perpetual Emotion" (2001) and a crossover homage to one of Brazil's great composers, "Flora sings Milton Nascimento" (2000). In 2002, during a residency at Ronnie Scott's in London, Purim and her husband Airto, collaborated with British producer Darren Allison and renowned flamenco guitarist Juan Martin on the latter's "Camino Latino" album. In 2005, she reunited with her old Return to Forever bandleader, Chick Corea. As of 2010, Purim is still actively touring.