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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Dog fennel produces beneficial effects by relaxing the brain. Whether taken in supplement or herbal form, dog fennel relaxes the mind. Many use the perennial as a mild sedative to ease the effects of depression or anxiety. As an herbal tea, dog fennel is also a simple cure for insomnia.