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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Melatonin for dogs. 1. Melatonin is a class of drug called a neuro-hormone, it has a number of potential veterinary uses such as sedative properties, may act as an anti-convulsant, and it can help regulate your dog's body rhythms and reproductive cycles.