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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Calming a Dog with Herbal Treatments. 1  1. Give the dog an herbal supplement orally. Lots of all-natural herbal supplements are available commercially, whether in pill form or in tinctures. 2  2. Administer valerian to calm an excitable dog. This is a sedative herb that is effective in treating excitability and dog anxiety.