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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
The drugs used to sedate a dog are very effective, so they require a prescription from a veterinarian and can only be administered by a veterinarian. 1  The two most common drugs used by veterinarians to calm dogs are acepromazine (PromAceÂ®), and diazepam (ValiumÂ®).