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(Potable bitters, or bitters you can drink on their own, like Italian amari, are a distinct category.) The Kitchn explains that bitters use high proof alcohol for maximum flavor extraction and preservation, and that for a neutral flavor, vodka and grain alcohol, like Everclear, are best.
So I use both spirit and liquor to refer to any unsweetened distilled alcoholic beverage: vodka, gin, brandy, whiskey, tequila, and the like. Liqueur, on the other hand, is used for sweetened distilled alcoholic beverages: pastis, triple sec, amari, Chartreuse, Benedictine, etc.