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Tomatillos can quickly go from being ripe to splitting their skins, and are over-ripe if they have turned a pale yellow. Fully ripe tomatillos are usually 1 to 2 inches in diameter, with a tangy to sweet flavor. Under-ripe tomatillos do not fill the paper husk, may appear slightly shriveled and taste somewhat sour.
Although they can be picked when green, their heat and flavor increases as they are allowed to mature and ripen to colors. Sweet Bell type peppers are can be harvested when firm and full size (at least 3 1/2 to 4 inches) but still green. If left to ripen, they may also turn red, yellow, orange, purple or even chocolate-colored depending on the cultivar. The less green you see, the sweeter the taste in both sweet and hot peppers.