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Smackover, Arkansas. Smackover is a small city in Union County, Arkansas, United States. According to Citydata.com, the 2014 population was at 1,790.
Smackoverâs existence is a result of one of the largest and most dramatic oil discoveries in the nation. Its sixty-eight-square-mile oil field led the nationâs oil output in the mid 1920s. Prior to the discovery of oil, economy in the area initially relied upon cotton and a successful timber industry due to the vast forests of southern Arkansas. Smackover is located about two- and- a- half hours from Little Rock.