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It depends on the type of paint used in the existing painting. If it is an oil painting, you will need to use oil based paint. If it is a water based medium, like acrylic, use a water based paint. Gesso will work well for this. It is inexpensive, opaque and will help level the texture of the existing painting. You may want to lightly sand the painting before painting over.
Mixing acrylic with watercolor. By mixing acrylic with watercolor, you can create paint with very unique qualities of color and opacity, that can be adjusted based on the ratio of the paint types and water. All you have to do is set up a palette with several colors of watercolor, and using a palette knife, mix them with a dab of acrylic.