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It depends on the type of paint used in the existing painting. If it is an oil painting, you will need to use oil based paint. If it is a water based medium, like acrylic, use a water based paint. Gesso will work well for this. It is inexpensive, opaque and will help level the texture of the existing painting. You may want to lightly sand the painting before painting over.
When it comes to dimensional work nothing beatsStudio High Viscosity acrylic paint, with its thick consistency and satin finish, it retains brush or spatula marks. Studio Fluid Acrylic, which is fluid with a satin finish, is suitable for detailed work. Applied with a brush, it can be used for fine, regular lines, glaze effects and watercolour effects. It is guaranteed free of environmentally harmful heavy metals. Colour Chart (pdf) Product Information (pdf)