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It depends on the type of paint used in the existing painting. If it is an oil painting, you will need to use oil based paint. If it is a water based medium, like acrylic, use a water based paint. Gesso will work well for this. It is inexpensive, opaque and will help level the texture of the existing painting. You may want to lightly sand the painting before painting over.
You can use acrylic paints and mediums to enhance your print, whether the image is photo based or fine art reproduction. By adding paint and/or mediums to your print, you can bring it to life with texture, glazes of colour, or bright brush strokes of paint.