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Making the world better, one answer at a time. I think both phosphorylases as well water molecules (hydrolysis) can break those P-O-P bonds in ATP.
Every time an ATP molecule is split for energy (by a water molecule...why we call it hydrolysis) it is broken down into an ADP and inorganic phosphate WITH the release of one hydrogen ion (another name for a hydrogen ion is a proton; the proton comes from the water molecule).