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Making the world better, one answer at a time. I think both phosphorylases as well water molecules (hydrolysis) can break those P-O-P bonds in ATP.
ATP to ADP-Energy Release. This is done by a simple process, in which one of the phosphate molecules is broken off, therefore reducing the ATP from 3 phosphates to 2, forming ADP (Adenosine Diphosphate after removing one of the phosphates {Pi}).