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Making the world better, one answer at a time. I think both phosphorylases as well water molecules (hydrolysis) can break those P-O-P bonds in ATP.
The bonds between the last 2 phosphates are high energy bonds. When ATP releases the terminal (end) phosphate, energy is released while forming a new compound ADP. ADP can be recycled by adding another phosphate (phosphorylation) to form ATP again. Cellular respiration is the process that allows this to occur.