On 1 September 1818, he established the Calcutta School Society'. He and Radhakanta Deb were secretaries of the society. He worked tirelessly to establish some schools to teach in English and Bengali, according to new methods of teaching, at such places as Thanthania, Kalitala and Arpuly.
Every day, he visited the schools and Hindu College and met almost every student. So great was his attachment and commitment to these students that it acted as a great inspiration of many of them. Some of the greatest names in subsequent years were all his students.