Much of the work of the society consisted of publishing chromolithographs of Italian art works, especially fresco paintings, of earlier centuries and raising public awareness for the preservation of these works. One of the people most responsible for furthering the goals of  the society was Henry Layard, who joined in 1852. Some of the other important early members were John Ruskin, Charles Thomas Newton, and Henry Liddell.
The society's work centered on publishing chromolithographs of Italian art, particularly frescoes from earlier centuries, to raise public awareness about preserving these works.  Henry Layard was a key figure in advancing the society's goals by joining in 1852. John Ruskin, Charles Thomas Newton, and Henry Liddell were among the other early members who contributed significantly.