Cambridgeshire police saw the Huracan model near to the force's base in Parkside, Cambridge, on Sunday.
The vehicle, which retails from about Â£180,000, was then photographed being towed away on a recovery truck.
In a tweet, its roads policing unit said: "Even Lamborghinis need insurance." It added: "He was stopped outside the station!"
An uninsured Lamborghini sports car was seized after being stopped outside a police station.