The total harmonic distortion (THD) index and its calculation methods are presented to calibrate the sinusoidal motion of the low-frequency angular acceleration rotary table (LFAART) and make up the incomprehensive evaluation based on the angular acceleration amplitude and frequency error indexes. The THD is calculated from two measurement schemes: a unique scheme combining the optical shaft encoder and the laser triangulation sensor and a regular scheme using the fiber optical gyroscope (FOG). An improved reversing moments recognition method is presented to upgrade the accuracy of solving the angular motion amplitude based on optical shaft encoder output. The field experiment shows that the difference in the THD values achieved using the combining scheme and FOG is within 0.11% when the signal-to-noise ratio of the FOG signal is higher than 7.7 dB, indicating the accuracy of the proposed methods and the feasibility of taking THD as the index.