AbstractIn the era of big data and artificial intelligence (AI), advanced data storage and processing technologies are in urgent demand. The innovative neuromorphic algorithm and hardware based on memristor devices hold a promise to break the von Neumann bottleneck. In recent years, carbon nanodots (CDs) have emerged as a new class of nano‐carbon materials, which have attracted widespread attention in the applications of chemical sensors, bioimaging, and memristors. The focus of this review is to summarize the main advances of CDs‐based memristors, and their state‐of‐the‐art applications in artificial synapses, neuromorphic computing, and human sensory perception systems. The first step is to systematically introduce the synthetic methods of CDs and their derivatives, providing instructive guidance to prepare high‐quality CDs with desired properties. Then, the structure–property relationship and resistive switching mechanism of CDs‐based memristors are discussed in depth. The current challenges and prospects of memristor‐based artificial synapses and neuromorphic computing are also presented. Moreover, this review outlines some promising application scenarios of CDs‐based memristors, including neuromorphic sensors and vision, low‐energy quantum computation, and human–machine collaboration.