Initial scientific discoveries towards modern-day laser peening began in the early 1960s as pulsed-laser technology began to proliferate around the world. In an early investigation of the laser interaction with materials by Gurgen Askaryan and E.M. Moroz, they documented pressure measurements on a targeted surface using a pulsed laser. The pressures observed were much larger than could be created by the force of the laser beam alone. Research into the phenomenon indicated the high-pressure resulted from a momentum impulse generated by material vaporization at the target surface when rapidly heated by the laser pulse. Throughout the 1960s, a number of investigators further defined and modeled the laser beam pulse interaction with materials and the subsequent generation of stress waves. These, and other studies, observed that stress waves in the material were generated from the rapidly expanding plasma created when the pulsed laser beam struck the target. Subsequently, this led to interest in achieving higher pressures to increase the stress wave intensity. To generate higher pressures it was necessary to increase the power density and focus the laser beam (concentrate the energy), requiring that the laser beam-material interaction occur in a vacuum chamber to avoid dielectric breakdown within the beam in air. These constraints limited study of high-intensity pulsed laser–material interactions to a select group of researchers with high-energy pulsed lasers.
In the late 1960s a major breakthrough occurred when N.C. Anderholm discovered that much higher plasma pressures could be achieved by confining the expanding plasma against the target surface. Anderholm confined the plasma by placing a quartz overlay, transparent to the laser beam, firmly against the target surface. With the overlay in place, the laser beam passed through the quartz before interacting with the target surface. The rapidly expanding plasma was now confined within the interface between the quartz overlay and the target surface. This method of confining the plasma greatly increased the resulting pressure, generating pressure peaks of , over an order of magnitude greater than unconfined plasma pressure measurements. The significance of Anderholm's discovery to laser peening was the demonstration that pulsed laser–material interactions to develop high-pressure stress waves could be performed in air, not constrained to a vacuum chamber.